Engineered 2D Materials: The heterostructure effect

Abstract

Observation of magnetic ordering in 2D layered materials at finite temperatures have drawn significant interest in recent years. Though Mermin-Wagner-Hohenburg theorem forbids long range ordering in 2D systems, anisotropy can lead to spin ordering at finite temperatures. One of such classes of 2D magnets explored recently is the transition metal phosphorus trisulphides (MPS3, M = Mn, Fe, and Ni) that hosts antiferromagnetic (AFM) ground state at low temperatures [1]. The AFM ground state exhibits different spin dimensionalities, (viz., n=1,2, and 3) due to the presence of an axial or planar anisotropy or in the absence of any anisotropic element [2] which may be described by the Ising (e.g., FePS3), XY (e.g.,
NiPS3), and Heisenberg (e.g., MnPS3) Hamiltonians, respectively [1]. Engineered heterostructures of magnetic layered materials with high spin-orbit coupled systems like topological materials has the potential to control the quantum interactions unravelling a variety of exotic phe...