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The role of coherence in quantum thermodynamics has been extensively studied in the recent years and it is now well-understood that coherence between different energy eigenstates is a resource independent of other thermodynamics resources, such as work. A fundamental remaining open question is whether the laws of quantum mechanics and thermodynamics allow the existence a "coherence distillation machine", i.e. a machine that, by possibly consuming work, obtains pure coherent states from mixed states, at a nonzero rate. This question is related to another fundamental question: Starting from many copies of noisy quantum clocks which are (approximately) synchronized with a reference clock, can we distill synchronized clocks in pure states, at a non-zero rate? In this paper we study quantities called "coherence cost" and "distillable coherence", which determine the rate of conversion of coherence in a standard pure state to general mixed states, and vice versa, in the context of quantum thermodynamics. We find that the coherence cost of any state (pure or mixed) is determined by its Quantum Fisher Information (QFI), thereby revealing a novel operational interpretation of this central quantity of quantum metrology. On the other hand, we show that, surprisingly, distillable coherence is zero for typical (full-rank) mixed states. Hence, we establish the impossibility of coherence distillation machines in quantum thermodynamics, which can be compared with the impossibility of perpetual motion machines or cloning machines. To establish this result, we introduce a new additive quantifier of coherence, called the "purity of coherence", and argue that its relation with QFI is analogous to the relation between the free and total energies in thermodynamics.

In general relativity, the picture of space–time assigns an ideal clock to each world line. Being ideal, gravitational effects due to these clocks are ignored and the flow of time according to one clock is not affected by the presence of clocks along nearby world lines. However, if time is defined operationally, as a pointer position of a physical clock that obeys the principles of general relativity and quantum mechanics, such a picture is, at most, a convenient fiction. Specifically, we show that the general relativistic mass–energy equivalence implies gravitational interaction between the clocks, whereas the quantum mechanical superposition of energy eigenstates leads to a nonfixed metric background. Based only on the assumption that both principles hold in this situation, we show that the clocks necessarily get entangled through time dilation effect, which eventually leads to a loss of coherence of a single clock. Hence, the time as measured by a single clock is not well defined. However, the general relativistic notion of time is recovered in the classical limit of clocks.